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y(in)n(teraction)f(p) r(oten)n(tials)h(and)g(coupling)f(matrix)h(elemen)n(ts)g(for)2042 3205 y(electronically)i(excited)h(states)f(at)h(surfaces)f(is)h(still)h (missing.)2042 3304 y(Once)25 b(they)h(b)r(ecome)g(a)n(v)-5 b(ailable,)25 b(a)g(realistic)g(description)g(of)h(re-)2042 3404 y(actions)k(with)h(electronic)g(transitions)e(at)i(surfaces)f (should)h(b)r(e)2042 3504 y(p)r(ossible.)2538 3784 y Fq(A)n(CKNO)n(WLEDGEMENTS)2125 4002 y Ft(W)-7 b(e)33 b(thank)f(E.)g(Kolo)r(dney)f(for)h(pro)n(viding)f(us)i(with)f(the)h (un-)2042 4101 y(published)i(data)g(of)g(the)g(I)2902 4113 y Fn(2)2974 4101 y Ft(disso)r(ciation)g(probabilit)n(y)f(in)h(the) 2042 4201 y(I)2072 4213 y Fn(2)2109 4201 y Ft(/diamond)f(scattering.)56 b(W)-7 b(e)35 b(also)f(are)f(grateful)h(that)h(Prof.)2042 4300 y(Kolo)r(dney)e(and)h(Prof.)56 b(Amira)n(v)34 b(gran)n(ted)f(the)i (p)r(ermission)e(to)2042 4400 y(include)28 b(this)g(unpublished)g(data) f(in)h(our)f(pap)r(er.)p 2042 4619 2043 4 v 2080 5053 a Fr([1])34 b(G.R.)22 b(Darling)f(and)g(S.)f(Hollo)n(w)n(a)n(y)-6 b(,)23 b(Rep.)d(Prog.)i(Ph)n(ys.)f Fq(58)p Fr(,)i(1595)2194 5144 y(\(1995\).)2080 5235 y([2])34 b(A.)26 b(Gro\031,)h(Surf.)f(Sci.)g (Rep.)f Fq(32)p Fr(,)h(291)h(\(1998\).)2080 5327 y([3])34 b(G.J.)27 b(Kro)r(es,)g(Prog.)g(Surf.)f(Sci.)g Fq(60)p Fr(,)g(1)g(\(1999\).)1946 5645 y Ft(8)p eop %%Page: 9 9 9 8 bop -112 -83 a Fr([4])35 b(B.N.J.)22 b(P)n(ersson)f(and)f(M.)h(P)n (ersson,)i(Surf.)e(Sci.)g Fq(97)p Fr(,)h(609)g(\(1980\).)-112 8 y([5])35 b(B.N.J.)i(P)n(ersson)f(and)f(M.)i(P)n(ersson,)i(Sol.)d (Stat.)g(Comm.)f Fq(36)p Fr(,)3 100 y(175)26 b(\(1980\).)-112 191 y([6])35 b(Y.)49 b(Huang,)55 b(C.T.)50 b(Rettner,)55 b(D.J.)50 b(Auerbac)n(h,)k(and)49 b(A.M.)3 282 y(W)-6 b(o)r(dtk)n(e,)25 b(Science)h Fq(290)p Fr(,)g(111)h(\(2000\).)-112 374 y([7])35 b(J.T.)46 b(Kindt,)k(J.C.)c(T)-6 b(ully)g(,)50 b(M.)c(Head-Gordon)f(and)g(M.)g(A.)3 465 y(Gomez,)26 b(J.)g(Chem.)f(Ph)n(ys.)h Fq(109)p Fr(,)g(3629)h(\(1998\).)-112 556 y([8])35 b(G.D.)26 b(Billing,)i(J.)e(Chem.)f(Ph)n(ys.)h Fq(112)p Fr(,)g(335)h(\(2000\).)-112 648 y([9])35 b(H.)26 b(Guo,)i(P)-6 b(.)27 b(Saalfrank,)h(and)f(T.)g(Seideman,)g(Prog.)h (Surf.)f(Sci.)3 739 y Fq(62)p Fr(,)f(239)h(\(1999\).)-150 830 y([10])35 b(J.)j(Str\177)-38 b(omquist)36 b(and)h(S.)g(Gao,)42 b(J.)c(Chem.)f(Ph)n(ys.)g Fq(106)p Fr(,)42 b(5751)3 922 y(\(1997\).)-150 1013 y([11])35 b(N.)26 b(Chakrabarti,)j(N.)d(Sath)n(y) n(am)n(urth)n(y)-6 b(,)24 b(and)j(J.W.)g(Gadzuk,)h(J.)3 1104 y(Ph)n(ys.)d(Chem.)g(A)h Fq(102)p Fr(,)g(4154)h(\(1998\).)-150 1196 y([12])35 b(T.)c(Kl)r(\177)-41 b(uner,)32 b(H.-J.)f(F)-6 b(reund,)31 b(V.)f(Staemmler)f(and)h(R.)g(Koslo\013,)3 1287 y(Ph)n(ys.)25 b(Rev.)g(Lett.)h Fq(80)p Fr(,)h(5208)g(\(1998\).) -150 1378 y([13])35 b(P)-6 b(.)25 b(Saalfrank,)i(Chem.)e(Ph)n(ys.)h Fq(193)p Fr(,)h(119)f(\(1995\).)-150 1469 y([14])35 b(P)-6 b(.)25 b(Saalfrank,)i(Surf)f(Sci..)g Fq(390)p Fr(,)h(1)f(\(1997\).)-150 1561 y([15])35 b(S.)25 b(Gao,)i(Ph)n(ys.)f(Rev.)f(B)h Fq(60)p Fr(,)g(15609)i(\(1999\).)-150 1652 y([16])35 b(A.)21 b(Gro\031,)j(S.)d(Wilk)n(e,)i(and)e(M.)h(Sc)n(he\017er,)g(Ph)n (ys.)f(Rev.)g(Lett.)h Fq(75)p Fr(,)3 1743 y(2718)27 b(\(1995\).)-150 1835 y([17])35 b(A.)25 b(Gro\031,)i(J.)g(Chem.)e(Ph)n(ys.)g Fq(110)p Fr(,)i(8696)g(\(1999\).)-150 1926 y([18])35 b(Z.S.)21 b(W)-6 b(ang,)23 b(G.R.)e(Darling)h(and)f(S.)g(Hollo)n(w)n(a) n(y)-6 b(,)23 b(Surf.)f(Sci.)f Fq(458)p Fr(,)3 2017 y(63)26 b(\(2000\).)-150 2109 y([19])35 b(A.)23 b(Gro\031)i(and)e(M.)i(Sc)n (he\017er,)f(Ph)n(ys.)f(Rev.)h(B)g Fq(61)p Fr(,)g(8425)i(\(2000\).)-150 2200 y([20])35 b(P)-6 b(.)25 b(P)n(ec)n(h)n(uk)l(as,)h(Ph)n(ys.)f(Rev.) g Fq(181)p Fr(,)i(166)g(\(1969\).)-150 2291 y([21])35 b(H.-D.)27 b(Mey)n(er)g(and)h(W.H.)f(Miller,)j(J.)e(Chem.)g(Ph)n(ys.)f Fq(70)p Fr(,)i(3214)3 2383 y(\(1979\).)-150 2474 y([22])35 b(M.F.)26 b(Herman,)f(J.)i(Chem.)e(Ph)n(ys.)g Fq(76)p Fr(,)i(2949)g(\(1982\).)-150 2565 y([23])35 b(M.F.)26 b(Herman,)f(J.)i(Chem.)e(Ph)n(ys.)g Fq(81)p Fr(,)i(754)f(\(1984\).)-150 2657 y([24])35 b(J.C.)27 b(T)-6 b(ully)g(,)25 b(J.)i(Chem.)e(Ph)n(ys.)g Fq(93)p Fr(,)i(1061)g(\(1990\).)-150 2748 y([25])35 b(D.F.)20 b(Cok)n(er)h(and)f(L.)h(Xiao,)h(J.)f(Chem.)f(Ph)n(ys.)g Fq(102)p Fr(,)i(496)g(\(1995\).)-150 2839 y([26])35 b(O.V.)24 b(Prezhdo)h(and)f(P)-6 b(.J.)25 b(Rossky)-6 b(,)24 b(J.)h(Chem.)f(Ph)n (ys.)h Fq(107)p Fr(,)g(825)3 2931 y(\(1997\).)-150 3022 y([27])35 b(M.S.)g(T)-6 b(opaler,)37 b(T.C.)f(Allison,)i(D.W.)c(Sc)n(h) n(w)n(enk)n(e,)i(and)e(D.G.)3 3113 y(T)-6 b(ruhlar,)26 b(J.)g(Chem.)f(Ph)n(ys.)h Fq(109)p Fr(,)g(3321)i(\(1998\).)-150 3205 y([28])35 b(A.)j(Danon)g(and)g(A.)h(Amira)n(v,)h(Ph)n(ys.)f(Rev.)f (Lett.)g Fq(61)p Fr(,)43 b(2961)3 3296 y(\(1988\).)-150 3387 y([29])35 b(C.)26 b(Bac)n(h)g(and)f(A.)h(Gro\031,)h(F)-6 b(arada)n(y)26 b(Discuss.)g Fq(117)p Fr(,)h(99)f(\(2000\).)-150 3479 y([30])35 b(W.)19 b(Brenig,)j(T.)d(Brunner,)i(A.)e(Gro\031,)j(and) c(R.)h(Russ,)i(Z.)e(Ph)n(ys.)g(B)3 3570 y Fq(93)p Fr(,)26 b(91)g(\(1993\).)-150 3661 y([31])35 b(S.)24 b(Hammes-Sc)n(hi\013er)e (and)i(J.C.)i(T)-6 b(ully)g(,)25 b(J.)g(Chem.)f(Ph)n(ys.)g Fq(101)p Fr(,)3 3753 y(4657)j(\(1994\).)-150 3844 y([32])35 b(D.)19 b(Kohen,)i(F.H.)f(Stillinger,)j(and)c(J.C.)j(T)-6 b(ully)g(,)20 b(J.)h(Chem.)e(Ph)n(ys.)3 3935 y Fq(109)p Fr(,)26 b(4713)h(\(1998\).)-150 4027 y([33])35 b(J.-Y.)22 b(F)-6 b(ang)21 b(and)h(S.)f(Hammes-Sc)n(hi\013er,)f(J.)j(Chem.)e(Ph)n (ys.)g Fq(110)p Fr(,)3 4118 y(11166)27 b(\(1999\).)-150 4209 y([34])35 b(W.)54 b(Gautsc)n(hi,)63 b Fs(Numeric)l(al)54 b(A)n(nalysis:)88 b(an)54 b(Intr)l(o)l(duction)p Fr(,)3 4301 y(Birkh\177)-38 b(auser,)26 b(Boston)h(\(1997\).)-150 4392 y([35])35 b(A.G.)27 b(Boriso)n(v,)h(V.)e(Sidis,)h(and)g(H.)f(Win)n (ter,)h(Ph)n(ys.)f(Rev.)g(Lett.)3 4483 y Fq(77)p Fr(,)g(1893)h (\(1996\).)-150 4575 y([36])35 b(G.R.)26 b(Darling,)i(Y.)e(Zeiri,)h (and)f(R.)g(Koslo\013,)h(F)-6 b(arada)n(y)26 b(Discuss.)3 4666 y Fq(117)p Fr(,)g(41)h(\(2000\).)-150 4757 y([37])35 b(M.I.)h(Landstrass)g(and)f(K.V.)g(Ra)n(vi,)j(Appl.)d(Ph)n(ys.)g(Lett.) h Fq(55)p Fr(,)3 4848 y(975)26 b(\(1989\).)-150 4940 y([38])35 b(F.)30 b(Maier,)i(M.)e(Riedel,)h(B.)f(Man)n(tel,)h(J.)g (Ristein,)g(and)e(L.)h(Ley)-6 b(,)3 5031 y(Ph)n(ys.)25 b(Rev.)g(Lett.)h Fq(85)p Fr(,)h(3472)g(\(2000\).)-150 5122 y([39])35 b(S.-T)-6 b(ong)24 b(Lee)g(and)f(G.)i(Apai,)f(Ph)n(ys.)g (Rev.)f(B)h Fq(48)p Fr(,)h(2684)h(\(1993\).)-150 5214 y([40])35 b(M.)25 b(Hand)e(and)h(J.)h(Harris,)g(J.)g(Chem.)f(Ph)n(ys.)g Fq(92)p Fr(,)h(7610)h(\(1990\).)-150 5305 y([41])35 b(A.)25 b(Gro\031)i(and)e(W.)h(Brenig,)h(Chem.)e(Ph)n(ys.)h Fq(177)p Fr(,)g(497)h(\(1993\).)-150 5396 y([42])35 b(A.)25 b(Gro\031)i(and)e (W.)h(Brenig,)h(Surf.)f(Sci.)g Fq(302)p Fr(,)g(403)h(\(1994\).)2042 -83 y([43])34 b(M.)27 b(Dohle)f(and)f(P)-6 b(.)26 b(Saalfrank,)g(Surf.) g(Sci.)g Fq(373)p Fr(,)h(95)f(\(1997\).)2042 8 y([44])34 b(K.P)-6 b(.)43 b(Hub)r(er)e(and)h(G.)g(Herzb)r(erg,)47 b(Constan)n(ts)c(of)g(Diatomic)2194 100 y(Molecules,)28 b(V)-6 b(an)25 b(Nostrand-Reinhold,)g(New)h(Y)-6 b(ork)25 b(\(1979\).)2042 191 y([45])34 b(L.D.)41 b(Landau)e(and)h(E.M.)h (Lifshitz,)k Fs(Quantum)c(Me)l(chanics,)2194 282 y(Non-r)l(elativistic) 23 b(The)l(ory)p Fr(,)f(P)n(ergamon)d(Press,)j(London)c(\(1958\).)2042 374 y([46])34 b(J.C.)28 b(T)-6 b(ully)g(,)25 b(F)-6 b(arada)n(y)26 b(Discuss.)g Fq(110)p Fr(,)h(407)g(\(1998\).)2042 465 y([47])34 b(E.)27 b(Kolo)r(dney)-6 b(,)25 b(priv)l(ate)g(comm)n (unication.)2042 556 y([48])34 b(R.B.)c(Gerb)r(er)f(and)g(R.)g(Elb)r (er,)i(Chem.)d(Ph)n(ys.)h(Lett.)g Fq(102)p Fr(,)i(466)2194 648 y(\(1983\).)2042 739 y([49])j(R.B.)c(Gerb)r(er)f(and)g(R.)g(Elb)r (er,)i(Chem.)d(Ph)n(ys.)h(Lett.)g Fq(107)p Fr(,)i(141)2194 830 y(\(1984\).)2042 922 y([50])j(J.W.)28 b(Gadzuk)d(and)h(S.)g(Hollo)n (w)n(a)n(y)-6 b(,)28 b(J.)f(Chem.)e(Ph)n(ys.)h Fq(84)p Fr(,)i(3502)2194 1013 y(\(1986\).)2042 1104 y([51])34 b(J.W.)27 b(Gadzuk,)f(Surf.)f(Sci.)h Fq(184)p Fr(,)h(483)g(\(1987\).) 1946 5645 y Ft(9)p eop %%Trailer end userdict /end-hook known{end-hook}if %%EOF